Probing inhomogeneous vibrational reorganization energy barriers of interfacial electron transfer

Article Abstract:

An atomic force microscopy (AFM) and confocal Raman microscopy study of the interfacial electron transfer of a dye-sensitization system has revealed the distribution of the mode-specific vibrational reorganization energies encompassing different local sites. The results demonstrate a significant step forward in characterizing the site-specific inhomogeneous interfacial charge-transfer dynamics.

Analysis, Electron transport, Atomic force microscopy

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Single-molecule triplet-state photon antibunching at room temperature

Article Abstract:

A single-molecule metal-to-ligand charge transfer (MLCT) dynamics of a ruthenium complex at room temperature is investigated. Using photon antibrunching measurement under continuous wave (CW) laser excitation, nonclassical photon statistics, and excitation power dependent measurements, a selective measure of the single-molecule MLCT state lifetime is achieved.

Primary nonferrous metals, not elsewhere classified, Primary Smelting and Refining of Nonferrous Metal (except Copper and Aluminum), Ruthenium, Ligands, Ligands (Chemistry), Chemical properties

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